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Journal Articles

Origin of Cs-bearing silicate glass microparticles observed during Fukushima accident and recommendations on nuclear safety

Hidaka, Akihide

Journal of Radioanalytical and Nuclear Chemistry, 332, p.1607 - 1623, 2023/03

 Times Cited Count:0 Percentile:0.01(Chemistry, Analytical)

no abstracts in English

Journal Articles

Clogging properties of HEPA filter induced by loading of soot from burned glove-box panel materials

Tashiro, Shinsuke; Ono, Takuya; Amano, Yuki; Yoshida, Ryoichiro; Watanabe, Koji*; Abe, Hitoshi

Nuclear Technology, 208(10), p.1553 - 1561, 2022/10

 Times Cited Count:1 Percentile:0.01(Nuclear Science & Technology)

To contribute to the confinement safety evaluation of the radioactive materials in the Glove box (GB) fire accident, combustion tests with the Polymethyl methacrylate (PMMA) and the Polycarbonate (PC) as typical panel materials for the GB have been conducted with a relatively large scale apparatus. As the important data for evaluating confinement safety, the release ratio and the particle size distribution of the soot generated from the burned materials were obtained. Furthermore, the rise of the differential pressure ($$Delta$$P) of the high efficiency particle air (HEPA) filter by the soot loading was also investigated. As results, the release ratio of the soot from the PC was about seven times as large as the PMMA. In addition, it was found that the behavior of the rise of the $$Delta$$P with soot loading could be represented uniformly regardless of kinds of combustion materials by considering effect of the loading volume of the soot particle in the relatively low loading region.

Journal Articles

Differential pressure changes of a high airflow-type HEPA filter during solvent fire in reprocessing facilities

Tashiro, Shinsuke; Uchiyama, Gunzo; Ono, Takuya; Amano, Yuki; Yoshida, Ryoichiro; Abe, Hitoshi

Nuclear Technology, 208(7), p.1205 - 1213, 2022/07

 Times Cited Count:0 Percentile:0.01(Nuclear Science & Technology)

A clogging behavior of a high-efficiency particulate air (HEPA) filter at solvent fire accidents for reprocessing facilities has been studied. In this study, the burning rates of 30% tri-butyl phosphate (TBP)/dodecane (DD) mixed solvent and DD solvent and the differential pressure ($$Delta$$P) of a high airflow typed HEPA filter applied in the actual facilities in Japan were measured. It was confirmed that the mainly burned was DD at the early stage of the mixed solvent burning and the TBP at the late stage. Furthermore, it was found that the $$Delta$$P rapidly rose at the late stage of the mixed solvent burning. The increase of the release ratio of the unburned particulate composition (TBP, its degraded solvent and inorganic phosphorus (P$$_{2}$$O$$_{5}$$)) was considered to contribute to the rapid rise. The correlating formulas with the $$Delta$$P and the mass of the loading particulates, except for the region of the rapid rise of $$Delta$$P, could be induced.

Journal Articles

Identification of carbon in glassy cesium-bearing microparticles using electron microscopy and formation mechanisms of the microparticles

Hidaka, Akihide

Nuclear Technology, 208(2), p.318 - 334, 2022/02

 Times Cited Count:6 Percentile:64.12(Nuclear Science & Technology)

The author previously proposed that the Cs bearing microparticle (Type A) may have been formed by melting and atomization of glass fibers (GF) of the HEPA filter in the SGTS due to flame and blast during the hydrogen explosion in Unit 3. If this hypothesis is correct, the Type A could contain or accompany carbon (C), that ignites spontaneously above 623 K, because of the limited time to be heated up, inclusion of C in the binder applied on the GF surface and closely located charcoal filter. As the previous studies did not focus on C, the present analyses were performed with EPMA whether the Type A contains C. The results showed that the Type A contained C originating from the binder, and non-spherical particles accompanied by the Type A and the film surrounding the Type A contained more C, which is thought to originate from the charcoal filter. These results cannot be explained by the other mechanisms proposed so far, and can be explained consistently by the author proposed hypothesis.

Journal Articles

Formation of Type A glassy cesium-bearing microparticles from HEPA filter materials in Unit 3 during Fukushima Dai-ichi NPS accident; From viewpoint of similarity in silicate glass composition

Hidaka, Akihide

Proceedings of 2021 International Congress on Advances in Nuclear Power Plants (ICAPP 2021) (USB Flash Drive), 10 Pages, 2021/10

Author recently proposed that the Type A glassy Cesium-bearing microparticles that were released during the Fukushima accident may have been formed by melting and atomization of glass fibers of the High Efficiency Particulate Air (HEPA) filter in the Stand-by Gas Treatment System (SGTS) line in Unit 3 during the hydrogen explosion. In the present study, the components of the Type A and glass fibers of HEPA filter were examined using EPMA. The results showed that the components of the Type A were almost the same as that of the glass fibers except for Cs, Fe, Sn, which are considered to have been contained in the in-vessel-derived particles. When the glass fiber was irradiated with the electron beam of the Electron Probe Micro Analyzer (EPMA) under vacuum condition, spherical particles of a few micro m size were formed that looked very similar to the Type A. These strongly suggest that the HEPA filter is Si source of the Type A.

Journal Articles

How the Cesium-bearing microparticles were generated?; Inference of an interdiscipinary researcher

Hidaka, Akihide

Nihon Genshiryoku Gakkai-Shi ATOMO$$Sigma$$, 63(9), p.679 - 680, 2021/09

no abstracts in English

Journal Articles

Formation mechanisms of insoluble Cs particles observed in Kanto district four days after Fukushima Daiichi NPP accident

Hidaka, Akihide

Journal of Nuclear Science and Technology, 56(9-10), p.831 - 841, 2019/09

AA2018-0262.pdf:0.88MB

 Times Cited Count:12 Percentile:79.53(Nuclear Science & Technology)

The insoluble Cs particles (Type A) were firstly observed in Tsukuba-city on the morning of March 15. The particles have been considered to be generated in RPV of Unit 2 by evaporation/condensation based on the measured $$^{134}$$Cs/$$^{137}$$Cs ratio and the core temperatures of each unit. However, the Type A particles with smaller diameter than the Type B particles of Unit 1 origin, are covered by almost pure silicate glass and have a trace of the quenching. This indicates that the particles could have been generated due to the melting of the HEPA filter in SGTS by the fire of H$$_{2}$$ detonation at Unit 3, and atomization followed by quenching of the molten materials by air blast of the explosion. Although the particles were mostly dispersed to the sea because of the wind direction, some of them deposited onto the lower elevation of R/B at Unit 3, could have been subsequently re-suspended and released into the environment, by the steam flow in the R/B caused by restart of the Unit 3 core cooling water injection at 2:30 of March 15.

Journal Articles

HEPA filter clogging and volatile material release under solvent fire accident in fuel reprocessing facility

Ono, Takuya; Watanabe, Koji; Tashiro, Shinsuke; Amano, Yuki; Abe, Hitoshi

Proceedings of 25th International Conference on Nuclear Engineering (ICONE-25) (CD-ROM), 7 Pages, 2017/07

After the Fukushima-Daiichi accident, countermeasures against the severe accident are newly required as regulatory items for nuclear facilities. Organic solvent fire in cell was defined as one of the accidents in the fuel reprocessing plant. When the solvent burns, aerosols including soot are released. The substances clog HEPA filters in the ventilation system and their breakthrough may happen because of differential pressure rising. Moreover, the fire can also release volatile radioactive gaseous species, which can pass through HEPA filters. These phenomena are important for evaluation of confinement capability of the facility and public exposure. We have investigated, in relating to the clogging behavior, release behavior of aerosols as well as of volatile materials from burnt solvent. In the presentation, we will report experimental data and evaluation results obtained from recent research.

JAEA Reports

Safety demonstration tests on thermal decomposition of nitrated solvent with nitric acid in nuclear fuel reprocessing plants (Contract research)

Tsukamoto, Michio; Takada, Junichi; Koike, Tadao; Watanabe, Koji*; Miyata, Teijiro*; Nishio, Gunji*; Murata, Mikio*; Uchiyama, Gunzo

JAERI-Tech 2001-031, 47 Pages, 2001/03

JAERI-Tech-2001-031.pdf:2.75MB

no abstracts in English

Journal Articles

Behavior of radioactive aerosols in cell-ventillation system in reprocessing plants

Murata, Mikio; Takada, Junichi; Tsukamoto, Michio

KURRI-KR-30, p.5 - 11, 1998/00

no abstracts in English

Journal Articles

Time dependency of HEPA filter performance during loading with liquid particles

; ; Ikezawa, Yoshio

Hoken Butsuri, 32(2), p.185 - 191, 1997/00

no abstracts in English

JAEA Reports

Safety demonstration tests on pressure rise in ventilation system and blower integrity of a fuel-reprocessing plant

Takada, Junichi; Suzuki, Motoe; Tsukamoto, Michio; Koike, Tadao; *

JAERI-Tech 96-054, 237 Pages, 1996/12

JAERI-Tech-96-054.pdf:6.22MB

no abstracts in English

JAEA Reports

Safety demonstration tests of air-ventilation system for the postulated explosive burning in a cell of fuel-reprocessing plant

Takada, Junichi; Suzuki, Motoe; Tsukamoto, Michio; Koike, Tadao; Nishio, Gunji

JAERI-Tech 95-024, 339 Pages, 1995/03

JAERI-Tech-95-024.pdf:7.99MB

no abstracts in English

Journal Articles

Contamination control, clearing and radiation monitoring in nuclear research facilities

Ikezawa, Yoshio

Saikin No Kenkyu Shisetsu, 0, p.304 - 311, 1995/00

no abstracts in English

JAEA Reports

Computer code TRANS-ACE predicting for fire and explosion accidents in nuclear fuel reprocessing plants

Abe, Hitoshi; Nishio, Gunji; Naito, Yoshitaka

JAERI-M 93-220, 107 Pages, 1993/11

JAERI-M-93-220.pdf:2.36MB

no abstracts in English

JAEA Reports

None

*;

PNC TN9410 93-282, 92 Pages, 1993/10

PNC-TN9410-93-282.pdf:2.29MB

None

Journal Articles

Air monitoring and control in nuclear facilities

Ikezawa, Yoshio

Kurin Tekunoroji, 3(4), p.41 - 45, 1993/04

no abstracts in English

JAEA Reports

Large-scale demonstration tests of solvent fire and boilover burning during the fire in fuel-reprocessing plant

Nishio, Gunji; Suzuki, Motoe; Takada, Junichi; Koike, Tadao; Tsukamoto, Michio

JAERI-M 93-019, 209 Pages, 1993/02

JAERI-M-93-019.pdf:3.99MB

no abstracts in English

Journal Articles

Fire behavior and filter plugging during a postulated solvent fire in the extraction process of a nuclear fuel reprocessing plant

Hashimoto, Kazuichiro; Nishio, Gunji; Soda, Kunihisa

Nuclear Technology, 101, p.218 - 226, 1993/02

 Times Cited Count:7 Percentile:60.37(Nuclear Science & Technology)

no abstracts in English

JAEA Reports

Demonstration test on the safety of a cell ventilation system during a hypothetical explosive burning in a fuel reprocessing plant

Suzuki, Motoe; Nishio, Gunji; Takada, Junichi; Tsukamoto, Michio; Koike, Tadao

JAERI 1328, 90 Pages, 1993/01

JAERI-1328.pdf:4.24MB

no abstracts in English

30 (Records 1-20 displayed on this page)